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Images can be added to imagelist during design time or run time. Adding during design time is very easy.Please verify
yourself.
If you want code to add images run time, I can help it. First image...

To add the first image to a button that is the code

Well, I got the answer.The correct code is as below

CComVariant vrIndex = 1;

m_pButton->put_Image(vrIndex );

I changed my code and then error message also changed
hr = m_pToolbar->put_ImageList(m_pImageList);// Added this line this time
hr = m_pButton->put_Image(vrImage);//I am getting error message...

I got the error description like this
"ImageList must be initialized before it can be used"
But how to correct?

//#import "c:\windows\SysWow64\mscomctl.ocx" raw_interfaces_only //in window7

using namespace MSComctlLib;
CComPtr<IButtons> pButtons;
CComPtr<IButton> pButton;...